An exact form for the time dependent resonance Raman kernel at finite temperature is derived under the assumption that the ground and excited state potential surfaces of the system are harmonic. The resultant expression can be evaluated by matrix algebra and Fourier transformed numerically to recover Raman scattering and excitation profiles.
|Original language||English (US)|
|Number of pages||9|
|Journal||The Journal of Chemical Physics|
|State||Published - Dec 1 1984|
ASJC Scopus subject areas
- Physics and Astronomy(all)
- Physical and Theoretical Chemistry